Please use this identifier to cite or link to this item: https://hdl.handle.net/11147/13247
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dc.contributor.authorYuan, Gangen_US
dc.contributor.authorJiang, Yuen_US
dc.contributor.authorWang, Xiaoen_US
dc.contributor.authorMa, Jiaojiaoen_US
dc.contributor.authorMa, Haoen_US
dc.contributor.authorWang, Xiangen_US
dc.contributor.authorYağmurcukardeş, Mehmeten_US
dc.contributor.authorHu, Shengen_US
dc.date.accessioned2023-03-20T12:12:51Z-
dc.date.available2023-03-20T12:12:51Z-
dc.date.issued2023-02-
dc.identifier.urihttps://doi.org/10.1021/acs.jpclett.2c03579-
dc.identifier.urihttps://hdl.handle.net/11147/13247-
dc.descriptionFunding text The authors acknowledge support from the National Key Research and Development Program of China (2019YFA0705400), the National Natural Science Foundation of China (21972121 and 22021001), the Fundamental Research Funds for the Central Universities (20720210017), and the BAGEP Award of the Science Academy with funding supplied by Sevinc-Erdal Inonu Foundation. Computational resources were partially provided by TUBITAK ULAKBIM, High Performance and Grid Computing Center (TR-Grid e-Infrastructure), and by the Flemish Supercomputer Center (VSC).en_US
dc.description.abstractBiological ion channels use both their sizes and residual groups to reject large ions and molecules and allow highly selective permeation of small species with similar sizes. To realize these properties in artificial membranes, the main challenge is the precise control of both the channel size and the interior at the nanoscale. Here we report the permeation of ions and molecules through interlayer channels in graphene-based laminar membranes. The amino groups decorated on channel walls are found to form hydrogen bond networks with intercalated water molecules, thus providing a highly stable laminate structure and a controlled channel size. Solutes with hydration diameters of >10 Å are precisely sieved out. Small species permeate through with selectivities of up to a few thousand, governed by their distinct electrical interactions with channels depending on the atomistic distance from the charged species to the channel walls. Our work offers important insights into manipulating channel structures for enhanced separation performance at the nanoscale.en_US
dc.language.isoenen_US
dc.publisherAmerican Chemical Societyen_US
dc.relation.ispartofJournal Of Physical Chemistry Lettersen_US
dc.rightsinfo:eu-repo/semantics/embargoedAccessen_US
dc.subjectGrapheneen_US
dc.subjectIonsen_US
dc.subjectArtificial membranesen_US
dc.subjectAmino groupen_US
dc.titleIon and molecule sieving through highly stable graphene-based laminar membranesen_US
dc.typeArticleen_US
dc.authorid0000-0002-1416-7990en_US
dc.institutionauthorYağmurcukardeş, Mehmeten_US
dc.departmentİzmir Institute of Technology. Photonicsen_US
dc.identifier.wosWOS:000936852100001 - WOS:000963930000001en_US
dc.identifier.scopus2-s2.0-85148095070en_US
dc.relation.publicationcategoryMakale - Uluslararası Hakemli Dergi - Kurum Öğretim Elemanıen_US
dc.identifier.doi10.1021/acs.jpclett.2c03579-
dc.identifier.pmid36815312-
dc.contributor.affiliationXiamen Universityen_US
dc.contributor.affiliationXiamen Universityen_US
dc.contributor.affiliationXiamen Universityen_US
dc.contributor.affiliationXiamen Universityen_US
dc.contributor.affiliationXiamen Universityen_US
dc.contributor.affiliationXiamen Universityen_US
dc.contributor.affiliation01. Izmir Institute of Technologyen_US
dc.contributor.affiliationXiamen Universityen_US
dc.relation.issn1948-7185en_US
dc.description.volume14en_US
dc.description.issue7en_US
dc.description.startpage1702en_US
dc.description.endpage1707en_US
item.openairetypeArticle-
item.openairecristypehttp://purl.org/coar/resource_type/c_18cf-
item.fulltextWith Fulltext-
item.languageiso639-1en-
item.cerifentitytypePublications-
item.grantfulltextembargo_20250301-
crisitem.author.dept04.04. Department of Photonics-
Appears in Collections:Photonics / Fotonik
PubMed İndeksli Yayınlar Koleksiyonu / PubMed Indexed Publications Collection
Scopus İndeksli Yayınlar Koleksiyonu / Scopus Indexed Publications Collection
WoS İndeksli Yayınlar Koleksiyonu / WoS Indexed Publications Collection
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